Mainly off the top of my head, from memory. I do have a couple of books on the He111, including a couple from the Osprey range, Kagero, and Squadron/Signal, plus general volumes, but as mentioned, my main interest is North West Europe, and with this aircraft it's for the BoB period.
From what I remember from the books, not much detail is given, in any of them, regarding the H21 and it's deployment, apart from being in Hungary with KG4 (One photo shows what appears to be a patchy snow camouflage over the basic scheme, which would suggest daylight ops), and the various texts move on to the H22 and other variants.
When I get a chance, if I find anything, I'll post it, but it might be some time before I can.